Gas Hydrate Equilibrium Measurements for Multi-Component Gas Mixtures and Effect of Ionic Liquid Inhibitors /

Bibliographic Details
Main Author: Othman, Enas Azhar (Author)
Other Authors: Castier, Marcelo (Thesis advisor), Atilhan, Mert (Thesis advisor)
Format: Thesis eBook
Language:English
Published: [College Station, Texas] : [Texas A & M University], [2015]
Subjects:
Online Access:Link to OAK Trust copy

MARC

Tag First Indicator Second Indicator Subfields
LEADER 00000cam a2200000Ki 4500
001 in00003485913
005 20151206125617.0
006 m fo d
007 cr unu||||||||
008 150202s2015 txu obm 000 0 eng d
035 |a (OCoLC)ocn902646949 
035 |a (OCoLC)902646949 
035 |a (TxCM)http://hdl.handle.net/1969.1/152653 
040 |a TXA  |b eng  |e rda  |e pn  |c TXA  |d UtOrBLW 
049 |a TXAM 
099 |a 2014  |a Thesis  |a 1969.1/152653 
100 1 |a Othman, Enas Azhar,  |e author. 
245 1 0 |a Gas Hydrate Equilibrium Measurements for Multi-Component Gas Mixtures and Effect of Ionic Liquid Inhibitors /  |c by Enas Aznar Othman. 
264 1 |a [College Station, Texas] :  |b [Texas A & M University],  |c [2015] 
300 |a 1 online resource. 
336 |a text  |b txt  |2 rdacontent 
337 |a computer  |b c  |2 rdamedia 
338 |a online resource  |b cr  |2 rdacarrier 
347 |a text file  |b PDF  |2 rda 
500 |a "Major Subject: Chemical Engineering." 
500 |a Includes vita. 
502 |b Master of Science  |c Texas A & M University  |d 2014  |o http://hdl.handle.net/1969.1/152653 
504 |a Includes bibliographical references. 
516 |a Text (Thesis) 
520 3 |a Qatar holds the world's third-largest proven reserves of natural gas at 885 trillion cubic feet according to a recent report. Because of its desert climate, gas hydrate formation may seem an unlikely event in Qatar. However, its natural gas reservoirs are located 80 km offshore, in the North Field, and the production of liquefied natural gas (LNG) depends on reliable flow from offshore wellheads to onshore processing facilities. Classical methods for inhibiting hydrate formation are used in order to prevent pipeline plugging but changing gas concentrations and operating conditions make flow assurance quite challenging in the North Field. Between 2008 and 2011, sudden temperature drops near gas pipelines caused various incidents of gas pipeline blockage by hydrates, with a loss of US$ 10 million per day due to lost production for almost 4 weeks. Such unplanned shut downs jeopardize the reliable export of LNG to end users. This work presents the recent investigation on synthetic multi-component gas mixtures whose compositions are typical of Qatari natural gases with initiatives aimed at helping producers minimize costs, optimize operations, and prevent interruption of gas flow in offshore drilling and production. In addition, it presents hydrate inhibition data from a newly commissioned micro bench top reactor, a high-pressure autoclave and a rocking cell. The conditions for hydrate formation for pure methane and carbon dioxide were also measured, for validation purposes. The measured data were compared with literature results and those of a commercial simulator, HydraFLASH®. Upon validation of the calibration data and determination of the apparatus uncertainty, results for hydrate formation equilibrium points for Qatari natural gas sample were collected and compared to HydraFLASH® predictions. Different percentages of 2-hydroxy-N,N,N-trimethylethanaminium chloride, also known as choline chloride ionic liquid, were used as hydrate inhibitor for the same gas mixture. The ionic liquid's inhibition performance was compared to that of classical thermodynamic inhibitors (e.g. methanol). Ionic liquid inhibition showed (0.7 - 1.8) °C and (2 - 2.6) °C shift in the hydrate equilibrium curve with 1 wt. % and 5 wt. % of choline chloride respectively. While the inhibition performance of 1 wt. % and 5 wt. % of methanol, obtained using HydraFLASH℗ʼ software, were 2.8 °C and 4.4 °C respectively.The electronic version of this dissertation is accessible from http://hdl.handle.net/1969.1/152653 
588 |a Description from author supplied metadata (automated record created 2015-01-09 15:05:21). 
650 4 |a Major Chemical Engineering. 
653 |a Natural gas hydrates 
653 |a ionic liquid inhibitors 
653 |a Choline chloride 
653 |a HydraFLASH 
700 1 |a Castier, Marcelo,  |e thesis advisor. 
700 1 |a Atilhan, Mert,  |e thesis advisor. 
710 2 |a Texas A & M University,  |e degree granting institution. 
856 4 0 |u http://hdl.handle.net/1969.1/152653  |z Link to OAK Trust copy  |t 0 
948 |a cataloged  |b h  |c 2015/2/2  |d o  |e spoltoratski  |f 12:57:11 pm 
994 |a C0  |b TXA 
999 |a MARS 
999 f f |s 757cb992-7503-384b-8152-717515e8fdaa  |i c2c3ee19-2fed-35d0-ac3d-fb2259d5d77d  |t 0 
952 f f |a Texas A&M University  |b College Station  |c Electronic Resources  |d Available Online  |t 0  |e 2014 Thesis 1969.1/152653  |h Other scheme 
998 f f |a 2014 Thesis 1969.1/152653  |t 0  |l Available Online