Sorption of polycyclic aromatic hydrocarbons to minerals and low-organic-carbon aquifer sediments /

(NOC) to mineral surfaces in low-organic-carbon soils

Bibliographic Details
Main Author: Grimaldi, Gabriel Orlando
Format: Thesis eBook
Language:English
Published: [Place of publication not identified] : [publisher not identified] ; 1999.
Subjects:
Online Access:Link to OAKTrust copy
Description
Summary:(NOC) to mineral surfaces in low-organic-carbon soils
aggregation on the type and amounts of surfaces
all minerals, except kaolinite, was highest when Cs
and a low-organic-carbon aquifer sediment. Pyrene was
and Cs) promoted pyrene sorption to vermiculite, where
and sediments remain unclear. The objectives of this
and the possible influence of coatings and particle
and untreated samples, suggesting that mineral
available for pyrene sorption.
cations and mineral surface chemistry on the sorption
coefficients of individual minerals weighted by their
confirming previous studies where surface area could
contribution to the total surface area. The calculated
controlling the sorption of nontoxic organic chemicals
describe their hardness or softness, some qualitative
difference may be caused by specific a-cation bonds
different minerals. Results show a significant effect
estimates of mineral composition in the sediment
exchange capacity of this mineral. Pyrene sorption to
formed between the aromatic [] electrons in pyrene
found between Kd values and cation properties that
including kaolinite, quartz, hematite, vermiculite,
isotherms for a11 minerals and sediment were linear.
Kd was the same order of magnitude as the measured
molecules and exchangeable cations On the mineral
not account for differences in Kd values. Pyrene
of polycyclic aromatic hydrocarbons (PAH) to minerals,
of the saturating cation on pyrene's K4 value. Na-
other minerals saturated with the same cations. This
pyrene sorption,
relationships were evident. Softer cations (e.g., Ba
research were to study the influence of exchangeable
Results show a strong influence of the mineral type on
saturated minerals sorbed more than the Mg-saturated
saturated the surface. Equilibrium sorption of pyrene
selected as representative PAH. Equilibrium sorption
sorption varied over one order of magnitude for the
surface. Although no quantitative correlation was
surfaces control pyrene sorption. A composite Kd value
the effect could be observed due to the higher cation
The molecular mechanisms and major geochemical factors ics.
to the aquifer sand was the same for peroxide-treated
value, which is reasonable given the semi-quantitative
values for all the cations tested. Cs- and Be-
vermiculite sorbed between 3 and 22 times more than
versions. Quartz and vermiculite showed the highest Kd
was calculated by addition of the distribution
Item Description:"Major subject: Geology".
Vita.
Physical Description:xi, 117 leaves : illustrations ; 28 cm.
Also available online.
Bibliography:Includes bibliographical references (leaves 63-68).