The vanadyl complex of N,N'-bis(2-mercaptoethyl)-1, 5-diazacyclooctane /

(bme-daco)VO, exhibits square-pyramidal geometry about the

Bibliographic Details
Main Author: Hatley, Michelle Lynn, 1971-
Format: Thesis eBook
Language:English
Published: [Place of publication not identified] : [publisher not identified] ; 1997.
Subjects:
Online Access:Link to OAKTrust copy
Description
Summary:(bme-daco)VO, exhibits square-pyramidal geometry about the
appears that the electron withdrawing capacity of the vanadyl
applications in the crude oil industry as well as in the
basal plane and the 0-atom at the apex. The vanadium atom
biological realm. The N2 S2 tetradentate ligand N,N'-bis(2-
characterization of (bme-daco)VO are discussed and the
complex is compared to other square-pyramidal systems of bme-
daco, including [Ga-C,12,. In light of the reactivity of the
daco)VO was examined and compared to the former complex. It
electrophiles; however, some reactivity was seen with
hydrogen peroxide and sulfur dioxide.
lies 0.66 A above the best N2S2 plane. The synthesis and
mercaptoethyl)-l@5-diazacyclooctane, H2-bme-daco, has been
nickel(II) analogue of (bme-daco)VO, the reactivity of (bme-
oxygen deactivates the thiolate sulfurs towards
shown to complex the vanadyl moiety. The resulting complex,
The chemistry of the divalent vanadyl cation, (VO)2 + , finds
vanadium atom with the donor atoms of the ligand forming the
Item Description:"Major subject: Chemistry".
In title, numerals are used.
Vita.
Physical Description:x, 52 leaves : illustrations ; 28 cm.
Also available online.
Issued also on microfiche from Lange Micrographics.
Bibliography:Includes bibliographical references.