Synthetic studies of 3-deoxy-D-manno-2-octulosonic acid (KDO), 3-deoxy-D-arabino-2-heptulosonic acid (DAH), and their 4-epimers through the radical chemistry of Barton esters /

The radical chemistry of thiohydroxamates (Barton esters) was

Bibliographic Details
Main Author: Liu, Wansheng
Format: Thesis Book
Language:English
Published: [Place of publication not identified] : [publisher not identified] ; 1997.
Subjects:
Online Access:http://proxy.library.tamu.edu/login?url=http://proquest.umi.com/pqdweb?did=739891171&sid=1&Fmt=2&clientId=2945&RQT=309&VName=PQD
Description
Summary:The radical chemistry of thiohydroxamates (Barton esters) was
applied to the synthesis of the higher monosaccharides 3-
deoxy-D-manno-2-octulosonic acid (KDO), 3-deoxy-D-arabino-2-
heptulosonic acid (DAH), and their 4-epimers starting from
commercial D-glucono-1,5-lactone and D-ribonolactone,
respectively. DAH was synthesized in a concise manner and
with good diastereoselectivity, for the first time, by
radical chemistry. The regeneration of the carbonyl group
from phenylhydrazones by oxidation with hypervalent
organoiodine reagents, benzeneseleninic anhydride (BSA), and
nickel peroxide was studied. a-Acetoxy and a-alkyloxy azo
compounds were synthesized by the oxidation of hydrazones
with hypervalent organoiodine reagents. From the oxidation
of 2-phenylhydrazono-,v-butyrolactone, a novel rearrangement
leading to hexahydro1,3-oxazine-2,4-dione derivatives was
discovered. The synthetic utility and radical mechanisms
of the oxidation of phenylhydrazones with BSA and nickel
peroxide were established. Numerous methods for the
conversion of N',Ndimethylhydrazides to carboxylicacids
were developed. 2-Mercaptopyridine and thiophenol were used
to manipulate the 2- and 3-positions of propionate esters.
Acrylamide proved to be an effective radical trap for carbon
radicals generated from Barton esters. By this radical
chemistry, homologation of carboxylic acids to primary
carboxamides and the synthesis of mesoionic compounds, namely
the anhydro-2-alkyl3-acyliminothiazolo[3,2-a]pyridinium
hydroxide derivatives, were achieved.
Item Description:Vita.
"Major Subject: Chemistry".
In title, numerals are used.
Physical Description:ix, 222 leaves : illustrations ; 28 cm.
Issued also on microfiche from University Microfilms Inc.
Bibliography:Includes bibliographical references: pages 203-219.